These inventories reside at Canadian Global Emissions
Interpretation Centre on the CGEIC
Web site.
This data set contains one file with annual anthropogenic SO2 data.
Documentation on this data set
Documentation on Annual SO2 and NOX
GEIA Document nox85yr1.1a1 so285yr1.1a1 03 Jan 95
so2&nox 1985 annual (1,000 kg) 1
Document file: so2nox1a1.txt
Carmen M.Benkovitz | Phone: (516)282-4135
Brookhaven National Laboratory | FAX: (516)282-2887
Bldg. 426, ECD | INTERNET: cmb@bnl.gov
PO Box 5000 | BITNET: cmb@bnl
Upton, NY 11973-5000 |
International Global Atmospheric Chemistry Programme
Global Emissions Inventory Activity (GEIA)
Anthropogenic SO2/NOx Emission Inventories Version 1A.1
April 12, 1995
Carmen M. Benkovitz
Department of Applied Science
Brookhaven National Laboratory
Upton, NY 11973, USA
This document briefly describes how Version 1A.1 of the GEIA
inventories of anthropogenic emissions of SO2 and NOx were compiled. A full
description of this work is being prepared for publication in a peer-reviewed
scientific journal. Until the article is published, please give the following
reference when you use the data:
Benkovitz, C.M., J. Dignon, J. Pacyna, T. Scholtz, L. Tarrasón, E.
Voldner and T.E. Graedel. Global Inventories of Anthropogenic Emissions of
SO2 and NOx, (in preparation).
Version 1A.1 corrects errors in the emissions of countries in
northeastern Europe present in the February release of Version 1A inventories.
Introduction.
Current activities of the Anthropogenic SO2/NOx Committee center
around the compilation of Version 1 of the GEIA inventories. These
inventories are based on the GEIA-specified 1o x 1o grid (lower left corner at
180oW/90oS, west to east and south to north), reflect 1985 emissions and
consist of two data sets: Version 1A inventories with annual emissions at one
level and Version 1B inventories with seasonal emissions, two vertical levels
defined at 100 m) and sectoral split information. Emissions totals across
both
inventories will agree. Work is being carried out in two complementary
working groups; Carmen Benkovitz, Brookhaven National Laboratory, Upton,
NY, USA heads the work on the annual inventories, Eva Voldner, Atmospheric
Environment Services, Canada and Trevor Scholtz, ORTECH International,
Canada, head the work on the seasonal inventories.
GEIA Standards.
The standard GEIA grid definition for emissions inventory was
selected at the First GEIA Workshop on Global Emissions Inventories, held in
Baltimore, MD on December 1-2, 1991: origin at 180oW, 90oS, 1o x 1o
resolution (i.e., 360 cells in the longitude direction, 180 cells in the latitude
direction). At the Second GEIA Workshop on Global Emissions Inventories,
held in Lillestrřm, Norway, June 22-24, 1992, 1985 was selected as the year for
the initial GEIA inventory of anthropogenic SO2 and NOx emissions. The
standard GEIA gridded population file was selected at the Third GEIA
Workshop on Global Emissions Inventories, Amersfoort, The Netherlands,
January 31 - February 2, 1993. The file selected was developed by Logan
(Jennifer Logan, Harvard University, manuscript in preparation, 1993) using
statistical data on national, state, and urban populations.
Inventories of Anthropogenic Emissions of SO2 and NOx, Version 1A.1.
The annual inventory for SO2 emissions compiled by Spiro et al,
(1992) was selected to provide the default emissions data for the GEIA SO2
inventories. Anthropogenic emissions in this inventory include emissions from
fossil fuel combustion and smelter operations. The Dignon (1992) inventory
for NOx emissions, which includes emissions from fuel combustion only, was
selected to provide the default emissions data for the GEIA NOx inventories.
Most current anthropogenic emissions data for different geographic
regions were solicited from local research groups. The following data have
been incorporated in the GEIA inventories.
The most comprehensive inventories of anthropogenic emissions of
SO2 and NOx for 1985 in the United States and Canada has been compiled by
the National Acid Precipitation Assessment Program, NAPAP, (Wagner et al.,
1986; Saeger et al., 1989). Version 2 of the NAPAP emissions inventories
were selected to replace values in the basic GEIA inventories for the U.S. and
Canada. Annual values for point sources were directly allocated to the GEIA
1o x 1o grid; the NAPAP spatial allocation file, which allocated population to
the NAPAP 20 km grid was used as the basis for the allocation of area sources
to the GEIA grid.
The most comprehensive inventories of European anthropogenic
emissions of SO2 and NOx compiled under a unified methodology have been
assembled by the Co-Operative Program for Monitoring and Evaluation of the
Long Range Transmission of Air Pollutants in Europe, EMEP, (Sandnes and
Styve, 1992) and by the UN/ECE CORINAIR project (Bouscaren, 1990).
Emissions for western Europe have been taken from the CORINAIR work; the
EMEP inventories supply the data for areas not covered by CORINAIR.
Anthropogenic emissions of SO2 and NOx for Australia were obtained
from F. Carnovale (1992), Australian Environment Protection Authority,
AEPA. Total emissions received were gridded to 1o x 1o; additional
information for point sources was also included. NOx data for some point
sources were missing from both files.
Anthropogenic emissions of SO2 and NOx for South Africa were
obtained from S.M Lloyd, South African Department of National Health and
Population Development, and R.K. Dutkiewicz, Energy Research Institute,
University of Capetown (personal communication, 1993). Sectors represented
included electric generation, synfuels, industry, metallurgy, mining,
agriculture, transport and domestic. Data received were gridded to 1o x 1o
GEIA grid.
Kato and Akimoto (1992) developed inventories of anthropogenic
emissions of SO2 and NOx for 251 Asian countries east of Afghanistan and
Pakistan for years 1975, 1980, 1985, 1986 and 1987. Transformation (electric
utilities, petroleum refineries, etc.), industrial, transportation and other sectors
are included in these inventories. Estimates are available on a province and
regional basis for China and India; on a country basis for all other countries.
Emissions for 1987 were apportioned to a 1ox1o grid by Akimoto and Narita [,
1994 #293]. The 1985 to 1987 ratio of emissions by country were calculated,
and the gridded 1987 emissions were scaled to 1985 values using these ratios.
Y. Tonooka (Y. Tonooka, Institute of Behavioral Sciences, Tokyo, Japan,
personal communication, 1993) developed an inventory of anthropogenic SO2
emissions for five Asian countries: Japan, China, North and South Korea and
Taiwan; emissions from this inventory replaced the Akimoto and Narita values
for these countries.
Table 1 summarizes the emissions from each of the inventories used.
Table 1. Summary of Emission Totals from the Inventories Used in the
Compilation of the GEIA V1A.1 of Anthropogenic Emissions of SO2 and NOx.
______________________________________________________
Reference SO2 NOx Notes
(Tg S)/y (Tg N)/y
______________________________________________________
Basic Inventory
Spiro 25.07 Non-indust
Dignon(global) 23.44
North America
NAPAP 12.30 6.24
USSR point sources
Pacyna 4.85 0.50 East of 60 deg. E
Europe, Mid. East, N. Africa
CORINAIR/EMEP 21.26 6.07 Russia to 60 deg. E
So. Africa
So. Africa 0.93 0.22
Australia
Australian EPA 0.81 0.21
Asia
Kato & Akimoto 13.04 4.20
5 Asian countries
Tonooka 10.49
______________________________________________________
The manuscript describing the work to develop the GEIA Version 1A
inventories of anthropogenic emissions of SO2 and NOx will be submitted for
publication in the NARE special issue of the Journal of Geophysical Research;
authors are Carmen Benkovitz, Brookhaven National Laboratory USA, Jane
Dignon, Lawrence Livermore National Laboratory, USA, Jozef Pacyna, NILU,
Norway, Trevor Scholtz, ORTECH International, Canada, Leonor Tarrasón,
Norwegian Meteorological Institute, Norway, Eva Voldner, Atmospheric
Environment Services, Canada, and T.E. Graedel, AT&T Bell Laboratories,
USA.
References
Bouscaren, R., Inventaire des Emissions de Polluants dans L'Atmosphere
dans La Communate Europeenne en 1985, CITEPA, 1990.
Carnovale, F., P. Alviano, C. Carvalho, G. Deitch, S. Jiang, D. Macaulay and
M. Summers, Air Emissions Inventory for the Port Phillip Control Region,
Clean Air, 26, 134-144, 1992.
Dignon, J., NOx and SOx Emissions from Fossil Fuels: A Global
Distribution, Atmos. Environ., 26A, 1157-1163, 1992.
Kato, N. and H. Akimoto, Anthropogenic Emissions of SO2 and NOx in
Asia: Emissions Inventories (plus errata), Atmos. Environ., 26A, 2997-3017,
1992.
Saeger, M., J. Langstaff, R. Walters, L. Modica, D. Zimmerman, D. Fratt, D.
Dulleba, R. Ryan, J. Demmy, W. Tax, D. Sprague, D. Mudgett and A.S.
Werner, The 1985 NAPAP Emissions Inventory (Version 2): Development of
the Annual Data and Modelers' Tapes, Rep. EPA-600/7-89-012a, U.S.
Environmental Protection Agency, Research Triangle Park, NC, 1989.
Sandnes, H. and H. Styve, Calculated Budgets for Airborne Acidifying
Components in Europe, 1985, 1986, 1987, 1988, 1989, 1990 and 1991,
Meteorological Synthesizing Centre - West. The Norwegian Meteorological
Institute, Oslo, Norway, 1992.
Spiro, P.A., D.J. Jacob and J.A. Logan, Global Inventory of Sulfur Emissions
with a 1o x 1o Resolution, J. Geophys. Res., 97, 6023-6036, 1992.
Wagner, J., R.A. Walters, L.J. Maiocco and D.R. Neal, Development of the
1980 NAPAP Emissions Inventory, U.S. Environmental Protection Agency,
Washington, DC, 1986.
1 Countries included: Afghanistan, Bangladesh, Brunei, Cambodia, China,
Hong Kong, India, Indonesia, Japan, N. Korea, S. Korea, Laos, Macao,
Malaysia, Maldivies, Mongolia, Myanmar, Nepal, Pakistan, Philippines,
Singapore, Sri Lanka, Taiwan.
1 Emissions from the following countries are not included in the total: Albania,
Australia, Austria, Belgium, Bulgaria, Canada, Czechslovakia, Denmark,
Finland, France, E. Germany, W. Germany, Greece, Hungary, Iceland, India,
Ireland, Italy, Japan, N. Korea, S. Korea, Liechtenstein, Luxemburg, Malta,
Netherlans, Norway, Poland, Portugal, Romania, Ussr/Total, Spain, Sweden,
Switzerland, Taiwan, U.K., U.S.A., Yugoslavia.
(last modified 02/28/05)